Regardless of the nether biome you are in, the ambience will always cycle through C418’s 4 songs. (Ballad of The Cats, Dead Voxel, Concrete Halls, and Warmth). Lena Raine’s 3 songs will not play for any reason.
MCPE-224561
Lena Raine’s Nether Music Does Not Play
Resolved
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This issue is being tracked at MCPE-219051.